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창의적인 신지식 창출과 산업계와의 협력적 네트워크 구축

HIGHLY CITED PAPERS (HCP)

  • 전임교원이 최근 5년간 출판한 논문 중, 연도별 카테고리별 피인용 상위 1%에 달성된 논문
  • 매월 1회 업데이트
Article
Reversible disorder-order transitions in atomic crystal nucleation
Author
Jeon, Sungho; Heo, Taeyeong; Hwang, Sang-Yeon; Ciston, Jim; Bustillo, Karen C.; Reed, Bryan W.; Ham, Jimin; Kang, Sungsu; Kim, Sungin; Lim, Joowon; Lim, Kitaek; Kim, Ji Soo; Kang, Min-Ho; Bloom, Ruth S.; Hong, Sukjoon; Kim, Kwanpyo; Zettl, Alex; Kim, Woo
Corresponding Author Info
Prof. Lee, Won Chul (기계공학과)
Professor
E-mail
이메일wonchullee@hanyang.ac.kr
Document Type
Source
Science 2021, 371, 6528, 498
Times Cited
18 (2022.1.5.)
External Information
https://www.science.org/doi/10.1126/science.aaz7555
Abstract
[History]
- 2021년 July/August부로, 이 highly cited paper 의 인용 횟수가 분야와 출판 연도에 대해 인용 빈도가 높은 임계값을 기반으로 Chemistry 학술 분야에서 상위 1%에 올랐습니다.

[Abstract]
Nucleation in atomic crystallization remains poorly understood, despite advances in classical nucleation theory. The nucleation process has been described to involve a nonclassical mechanism that includes a spontaneous transition from disordered to crystalline states, but a detailed understanding of dynamics requires further investigation. In situ electron microscopy of heterogeneous nucleation of individual gold nanocrystals with millisecond temporal resolution shows that the early stage of atomic crystallization proceeds through dynamic structural fluctuations between disordered and crystalline states, rather than through a single irreversible transition. Our experimental and theoretical analyses support the idea that structural fluctuations originate from size-dependent thermodynamic stability of the two states in atomic dusters. These findings, based on dynamics in a real atomic system, reshape and improve our understanding of nucleation mechanisms in atomic crystallization.
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