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창의적인 신지식 창출과 산업계와의 협력적 네트워크 구축

HIGHLY CITED PAPERS (HCP)

  • 전임교원이 최근 5년간 출판한 논문 중, 연도별 카테고리별 피인용 상위 1%에 달성된 논문
  • 매월 1회 업데이트
SCIE Article
Ampere-hour-scale zinc-air pouch cells
Author
Shinde, SS; Jung, JY; Wagh, NK; Lee, CH; Kim, DH; Kim, SH; Lee, SU; Lee, JH
Corresponding Author Info
Prof. Lee, Jung-Ho (재료화학공학과 이정호 교수)
Professor
E-mail
이메일sa5353@hanyang.ac.kr
Document Type
Source
NATURE ENERGY 2021. 6.
Times Cited
46 (2022.09.28.)
External Information
10.1038/s41560-021-00807-8
Abstract
[History]
- 1월/2월 2022부로, 이 인용 빈도가 높은 논문의 인용 횟수가 분야와 출판 연도에 대해 인용 빈도가 높은 임계값을 기반으로 Materials Science 관련 학술 분야에서 상위 1%에 올랐습니다.

[Abstract]
All-solid-state zinc-air pouch cells promise high energy-to-cost ratios with inherent safety; however, finding earth-abundant high power/energy cathodes and super-ionic electrolytes remains a fundamental challenge. Here we present realistic zinc-air pouch cells designed by the (101)-facet copper phosphosulfide [CPS(101)] as a cathode as well as anti-freezing chitosan-biocellulosics as super-ionic conductor electrolytes. The proposed CPS(101) exhibits trifunctional activity and stability (>30,000 cycles) towards reversible oxygen reactions and hydrogen evolution reactions, outperforming commercial Pt/C and RuO2. Furthermore, hydroxide super-ion conductors utilizing polymerized chitosan-biocellulosics reveal exceptional conductivity (86.7 mS cm(-1) at 25 degrees C) with high mechanical/chemical robustness. High cell-level energy densities of 460 Wh kg(cell)(-1)/1,389 Wh l(-1) are normally measured in pouch cells (1 Ah) with a cycle lifespan of 6,000/1,100 cycles at 25 mA cm(-2) for 20/70% depths of discharge, and the highest densities we could achieve were 523 Wh kg(cell)(-1)/1,609 Wh l(-1). Flexible pouch cells operate well at rates of 5-200 mA cm(-2) over a broad temperature range of -20 to 80 degrees C. Zinc-air batteries are viewed as a sustainable storage technology, but their commercialization requires a genuine performance leap forwards from the laboratory scale. Here the authors report a cell-level design and demonstrate an ampere-hour pouch cell with exceptionally high energy density and cycle lifespan.
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