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창의적인 신지식 창출과 산업계와의 협력적 네트워크 구축

HIGHLY CITED PAPERS (HCP)

  • 전임교원이 최근 5년간 출판한 논문 중, 연도별 카테고리별 피인용 상위 1%에 달성된 논문
  • 매월 1회 업데이트
SCIE Article
In-situ reconstructed Ru atom array on alpha-MnO2 with enhanced performance for acidic water oxidation
Author
Lin, Chao; Li, Ji-Li; Li, Xiaopeng; Yang, Shuai; Luo, Wei; Zhang, Yaojia; Kim, Sung-Hae; Kim, Dong-Hyung; Shinde, Sambhaji S.; Li, Ye-Fei; Liu, Zhi-Pan; Jiang, Zheng; Lee, Jung-Ho
Corresponding Author Info
Prof. Lee, Jung-Ho (재료화학공학과 이정호 교수)
Professor
E-mail
이메일jungho@hanyang.ac.kr
Document Type
Source
NATURE CATALYSIS 2021, 4 1012-1023
Times Cited
234 (2024.01.31.)
External Information
http://dx.doi.org/10.1038/s41929-021-00703-0
Abstract
- 9월/10월 2022부로, 이 인용 빈도가 높은 논문의 인용 횟수가 분야와 출판 연도에 대해 Chemistry 관련 학술 분야에서 상위 1%에 올랐습니다.
<Abstract>
The development of acid-stable oxygen evolution reaction electrocatalysts is essential for high-performance water splitting. Here, we report an electrocatalyst with Ru-atom-array patches supported on alpha-MnO2 (Ru/MnO2) for the oxygen evolution reaction following a mechanism that involves only *O and *OH species as intermediates. This mechanism allows direct O-O radical coupling for O-2 evolution. Ru/MnO2 shows high activity (161 mV at 10 mA cm(-2)) and outstanding stability with small degradation after 200 h operation, making it one of the best-performing acid-stable oxygen evolution reaction catalysts. Operando vibrational and mass spectroscopy measurements were performed to probe the reaction intermediates and gaseous products for validating the oxygen evolution reaction pathway. First-principles calculations confirmed the cooperative catalysis mechanism with a reduced energy barrier. Time-dependent elemental analysis demonstrated the occurrence of the in-situ dynamic cation exchange reaction during the oxygen evolution reaction, which is the key for triggering the reconstruction of Ru atoms into the ordered array with high durability.
Web of Science Categories
Chemistry
Funding
Language
English
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